There are many huge PSRAM chips on the market, the problem is, the larger ones are all xSPI (8 lanes or more) and not compatible with the QSPI (4 lanes) implementation on Teensy 4.1., so a simple footprint adapter could not thelp.
I've looked it up and checked several dozens of datasheets, but there is actually only the IPUS IPS6404LSQ / ESP PSRAM64H and relabels left for use.